Note: When clicking on a Digital Object Identifier (DOI) number, you will be taken to an external site maintained by the publisher.
Some full text articles may not yet be available without a charge during the embargo (administrative interval).
What is a DOI Number?
Some links on this page may take you to non-federal websites. Their policies may differ from this site.
-
Abstract Topological magnons give rise to possibilities for engineering novel spintronics devices with critical applications in quantum information and computation, due to their symmetry-protected robustness and low dissipation. However, to make reliable and systematic predictions about the material realization of topological magnons has been a major challenge, due to the lack of neutron scattering data for most materials and the absence of reliable ab initio calculations for magnons. In this work, we significantly advance the symmetry-based approach for identifying topological magnons through developing a fully automated algorithm, utilizing the theory of symmetry indicators, that enables a highly efficient and large-scale search for candidate materials hosting perturbation-driven topological magnons. This progress not only streamlines the discovery process but also expands the scope of materials exploration beyond previous manual or traditional approaches, offering a powerful tool for uncovering novel topological phases in magnetic systems. Performing a large-scale search over all 1649 magnetic materials in the Bilbao Crystallographic Server (BCS) with a commensurate magnetic order, we discover 387 perturbation-induced topological magnon materials, significantly expanding the pool of topological magnon materials and showing that more than 23% of all commensurate magnetic compounds in the BCS database are topological. We further discuss examples and experimental accessibility of the candidate materials, shedding light on future experimental realizations of topological magnons in magnetic materials. We provide anopen-source programthat checks the symmetry-enforced magnon band topology of any commensurate magnetic structure upon perturbations and allows researchers to reproduce our results.more » « less
-
Abstract CrxPt1−xTe2is a recently developed van der Waals magnetic alloy noted for its stability under ambient conditions. Here, we report the emergence of an exchange bias effect in CrxPt1−xTe2, without typical exchange bias sources such as an adjacent antiferromagnetic layer. We find that the exchange bias is present forx = 0.45 and absent forx = 0.35, which is correlated to the presence of a Cr modulation where the Cr concentration alternates each vdW layer (modulation period of 2 layers) forx ≥ 0.4. We perform Monte Carlo simulations utilizing exchange parameters from first-principles calculations, which recreate the exchange bias in hysteresis loops of Cr0.45Pt0.55Te2. From our simulations, we infer the source of exchange bias to be magnetic moments locked into free energy minima that resist magnetization reversal. This work presents a way to introduce desirable magnetic properties to van der Waals magnets.more » « less
-
Two-dimensional (2D) materials have drawn immense interests in scientific and technological communities, owing to their extraordinary properties and their tunability by gating, proximity, strain and external fields. For electronic applications, an ideal 2D material would have high mobility, air stability, sizable band gap, and be compatible with large scale synthesis. Here we demonstrate air stable field effect transistors using atomically thin few-layer PdSe2 sheets that are sandwiched between hexagonal BN (hBN), with large saturation current > 350 μA/μm, and high field effect mobilities of ~ 700 and 10,000 cm2/Vs at 300 K and 2 K, respectively. At low temperatures, magnetotransport studies reveal unique octets in quantum oscillations that persist at all densities, arising from 2-fold spin and 4-fold valley degeneracies, which can be broken by in-plane and out-of-plane magnetic fields toward quantum Hall spin and orbital ferromagnetism.more » « less
-
Abstract The exploration of quantum materials in which an applied thermo/electrical/magnetic field along one crystallographic direction produces an anisotropic response has led to unique functionalities. Along these lines, KMgBi is a layered, narrow gap semiconductor near a critical state between multiple Dirac phases due to the presence of a flat band near the Fermi level. The valence band is highly anisotropic with minimal cross‐plane dispersion, which, in combination with an isotropic conduction band, enables axis‐dependent conduction polarity. Thermopower and Hall measurements indicate dominant p‐type conduction along the cross‐plane direction, and n‐type conduction along the in‐plane direction, leading to a significant zero‐field transverse thermoelectric response when the heat flux is at an angle to the principal crystallographic directions. Additionally, a large Ordinary Nernst effect (ONE) is observed with an applied field. It arises from the ambipolar term in the Nernst effect, whereby the Lorentz force on electrons and holes makes them drift in opposite directions so that the resulting Nernst voltage becomes a function of the difference between their partial thermopowers, greatly enhancing the ONE. It is proven that axis‐dependent polarity can synergistically enhance the ONE, in addition to leading to a zero‐field transverse thermoelectric performance.more » « less
An official website of the United States government
